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| REACTION KINETICS AND THE DEVELOPMENT OF CATALYTIC PROCESSES, 122
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Proceedings of the International Symposium, Brugge, Belgium, April 19-21, 1999
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Edited By
G.F. Froment, Laboratorium voor Petrochemische Techniek, Universiteit Gent, Ghent, Belgium
K.C. Waugh, Department of Chemistry, UMIST, Manchester, UK
Included in series
Studies in Surface Science and Catalysis, 122
Description
The symposium "Reaction Kinetics and the Development of Catalytic Processes" is the continuation of the very successful International
Symposium "Dynamics of Surfaces and Reaction Kinetics in Heterogeneous Catalysis", held in September 1997 in Antwerp, Belgium. These
proceedings contain a unique series of top level plenary lectures mainly focused on
• the dynamics of catalytic surfaces
•
the interaction of the reacting molecules with the solid catalyst
• the elementary steps of reaction pathways and molecular kinetics.
Surface
science techniques, molecular modeling, transient kinetic studies, sophisticated and specific reactors are included to a growing extent
in the kinetic modeling and the development of catalytic processes. How this is practiced today and how it will evolve in the coming
years, and what benefit can be expected for a more fundamentally based approach is the aim of the symposium.
Contents
Preface.
Keynotes.
Catalysis from first principles (J.K. Norskov).
Complexities and dynamics of the enantioselective
active site in heterogeneous catalysis (R. Raval, C.J. Baddeley, S. Haq, S. Louafi, P. Murray, C. Muryn, M. Ortega Lorenzo, J. Williams).
Intrinsic activities and pore diffusion effect in hydrocarbon cracking in steamed Y zeolite (H.H. Kung).
Internal reforming in solid
oxide fuel cells (R.M. Ormerod).
Microchemical reactors for heterogeneously catalyzed reactions (D. Hönicke).
Transient
Studies.
Novel frequency response techniques for the study of kinetics in heterogeneous catalysis (M. Cavers, J.M. Davidson,
I.R. Harkness, G.S. McDougall, L.V.C. Rees).
Reactivity of novel metal substituted heteropolyacid catalysts using steady-state and transient
response kinetics (H.T. Randall, P.L. Mills, K. Kourtakis).
Use of isotopic transient methods for mechanistic analysis of ethylene hydroformylation
over 4 wt% Rh/SiO2 catalyst (S.S.C. Chuang, S.A. Hedrick, M.A. Brundage).
CO oxidation over a supported Pt catalyst: transient
kinetics using temporal analysis of products (TAP) (A.H.J. Colaris, J.H.B. Hoebink, J.C. Schouten).
Transient kinetics of ethylene and
carbon monoxide oxidation for automotive exhaust gas catalysis: experiments and modeling (J.M.A. Harmsen, J.H.B. Hoebink, J.C. Schouten).
Dynamics of NO adsorption and transformation over supported Pt catalysts for the treatment of lean burn engine emissions (G.E. Arena,
A. Bianchini, G. Centi, F. Vazzana, P. Vitali).
Effect of catalyst deactivation on the dynamics of cyclic reactive processes (D.O. Borio,
N.S. Schbib, J.E. Gatica).
Propyne hydrogenation over a silica-supported platinum catalyst studied under transient conditions (D.R. Kennedy,
B. Cullen, D. Lennon, G. Webb, P.R. Dennison, S.D. Jackson).
A TAP reactor investigation of the oxidative dehydrogenation of propane
over a V/MgO catalyst: experiment and modeling (Y. Schuurman, T. Décamp, J.C. Jalibert, C. Mirodatos).
Transient behavior of an
industrial acetylene converter (N.S. Schbib, A.F. Errazu, J.A. Porras).
Modeling of alkane dehydrogenation under transient and steady
state conditions over a chromia catalyst using isotopic labelling (S.D. Jackson, J. Grenfell, I.M. Matheson, G. Webb).
The development
of a model capable of predicting diesel lean NOx catalyst performance under transient conditions (G.P. Ansell et al.).
Dynamics
of Surfaces.
Monte Carlo and lattice-gas studies of the kinetics of hydrocarbon hydrogenation reactions (A.S. McLeod, L.F. Gladden).
Time distribution of adsorption energies, local monolayer capacities, local isotherms and energy distribution functions on catalytic
surfaces (Ch. Abatzoglou, N.A. Katsanos, A. Kalantzopoulos, F. Roubani-Kalantzopoulou).
Molecular dynamical studies of the mobility of
benzene and water on silica surfaces: correlation with the influence of surface chemistry and morphology (S.P. Rigby, L.F. Gladden).
Experimental study of reaction instability and oxcillatory behavior during CO oxidation over Pd supported on glass fiber catalysts (I.Yuranov,
L. Kiwi-Minsker, V. Barelko, A. Renken).
Enhancement of selective conversion in spatially patterned reactors (A.S. Côté,
W.N. Delgass, D.Ramkrishna).
Novel Reactors.
A novel laboratory reactor for gas-phase transient kinetics based on time-of-flight
and quadrupole mass spectroscopy (H.T. Randall, P.L. Mills, J.S. McCracken).
Development of new photo-catalytic methods and reactors
for waste water treatment (A. Starosud, A. Bhargava, C.H. Langford, A. Kantzas).
An integrated dehydrogenation-hydrogenation membrane
reactor for the simultaneous production of styrene and cyclohexane (T.M. Moustafa, I. Ashour, S.S. Elnashaie).
A simple and flexible
micro reactor for investigations of heterogeneous catalytic gas phase reactions (G. Veser, G. Friedrich, M. Freygang, R. Zengerle).
The
use of a catalytic wall reactor for studying highly exothermic reactions (B. Amon, E. Klemm, G. Emig).
A novel reactor to activate chromium-catalysts
(H. Schönfelder, M. Kämmerer, W. de Lange).
Kinetic Modeling.
Kinetics and reactor simulation for polyethoxylation
and polyproproxylation reactions (E. Santacesaria, M. Di Serio, P. Iengo).
On the use of response reactions in the kinetic modeling of
complex heterogeneous catalytic reactions (I. Fishtik, R. Datta).
Kinetic effects of chemical modifications of PMO12 catalysts
for the selective oxidation of isobutane (M. Sultan, S. Paul, D. Vanhove).
Kinetic based deactivation modeling of an isothermal propane
dehydrogenation reactor (E.H. Stitt, S.D. Jackson, F.King).
Development of kinetic models for reactions of light hydrocarbons over ZSM-5
catalysts. Experimental studies and kinetic modeling of ethene transformation and deactivation of HZSM-5 catalyst (D.B. Lukyanov).
Two-dimensional
reactor modeling of the pure dehydrogenation of methanol to formaldehyde (S. Ruf, S. Schunk, G. Emig, Th. Weber, S. Braun, G. Brenner,
F. Durst).
Kinetic modeling of enzymatic chiral resolution of (±)2-methyl butyric acid (R. García, M. Martínez,
D. García, J. Aracil).
Regioselective synthesis of monoglycerides. Kinetic modeling (T.García, M. Martínez, D.
García, J. Aracil).
Kinetic modeling of paraffins hydrocracking based upon elementary steps and the single event concept (G. Martens,
G.F. Froment).
A comparative kinetic study of CH4 oxidation by NiO/Al2O3, Pt/Al2O3
and NiO-Pt/Al2O3 catalysts (T.-N. Angelidis, V. Tzitzios).
Catalysis in Processes.
Kinetic and
mass-transfer effects in the hydrogenation of xylose to xylitol (J.-P. Mikkola, T. Salmi, R. Sjöholm).
Methylation of biphenyl over
zeolite H-ZSM-5 in gas phase with methanol in presence of water: effect of the catalyst impregnation by tetraethyl orthosilicate (S.
Dubuis, R. Doepper, A. Renken).
Kinetics and mechanism studies of the catalytic dehydrogenation of isobutane on platinum-indium catalyst
(D. Casanave, K. Fiaty, J.A. Dalmon, M. Forrisier).
Synthesis of ethylbenzene from diethylbenzenes in the presence of benzene using triflic
acid as catalyst (M.C. Al-Kinany, S.H. Al-Khowaiter).
Elementary steps of reaction pathway in the pilot plant photomineralisation of
s-triazines on to photocatalytic membranes immobilising titanium dioxide and promoting photocatalysts (A. Moroni, I.R. Bellobono, B.M.
Gawlik).
Methane oxidation over supported nickel catalysts (A.M. Diskin, R.H. Cunningham, R.M. Ormerod).
Posters.
Novel
sensor for studying the transient behaviour of an iron antimonate partial oxidation catalyst (D.Barth, M. Sahibzada, I.S. Metcalfe).
Chemical equilibria in direct synthesis of dimethyl ether (M. Grzesik, J. Skrzypek).
Thermodynamics and kinetics of the synthesis of
higher aliphatic alcohols (M. Grzesik, M. Kulawska, J. Skrzypek, M. Witczak).
Kinetics of esterification of acrylic acid with C3
and C4 aliphatic alcohols in the presence of sulfuric acid as a catalyst (M. Grzesik, J.Skrzypek, M. Witczak).
Hydrogenation
of carbonaceous adsorbed species formed during the CO/H2 reaction on a Ru/Al2O3 catalyst: experiment
and kinetic modeling (H. Ahlafi, M. Nawdali, D. Bianchi).
Application of the continuous two impinging streams reactors in chemical absorption
(M. Sohrabi, A.M. Jamshidi).
A kinetic study of heck reaction of iodobenzene and methyl acrylate using homogeneous Pd/TPP catalyst (F.-G.
Zhao, B.M. Bhanage, M. Shirai, M. Arai).
Kinetic and catalytic aspects in the synthesis of polyethylene terephtalate (PET), also through
the use of model molecules (B. Apicella, E. Santacesaria, M. Di Serio).
H/D isotopic exchange between oxide surface and spiltover hydrogen
on nickel supported catalysts (V. Almasan, M. Lazar, P. Marginean).
Transient studies of adsorption kinetics (J. Kanervo, L.B. Backman,
A.O.I. Krause, S.-L. Jämsä-Jounela).
Modeling the voltammetric behaviour of cobalt cations inside zeolites (M.A.N. Lemos, P.
Sousa, F. Lemos, A.J.L. Pombeiro, F. Ramôa Ribeiro).
Modeling transient tracer studies of complex activation mechanisms of two-atom
labelled molecules (A.A. Shestov, R. Burch, J.A. Sullivan, V.S.Muzykantov).
Preparation of ZSM-5 zeolite film on metal support (A. Brehm,
U. Antons, A. Bekurdts).
A steady state isotopic transient kinetic analysis of NO reduction over Pt/SiO2 under lean burn conditions
(A.A. Shestov, R. Burch, J.A. Sullivan).
Modeling the dynamics of the surface of a carbon (C. Palma, I. Santos Silva, F. Lemos, L. Sousa
Lobo).
Investigation of isomerization kinetics of m-xylene over zeolite based catalysts (O. Akpolat, G. Gündüz).
Author
Index.
| Bibliographic details |
Hardbound, 0 pages, publication date: MAR-1999
ISBN-13: 978-0-444-50073-1
ISBN-10: 0-444-50073-1
Imprint: ELSEVIER
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