Nonlinear Optical Properties of Organic Molecules and Crystals V1 - 1st Edition - ISBN: 9780121706111, 9780323148153

Nonlinear Optical Properties of Organic Molecules and Crystals V1

1st Edition

Editors: D.S. Chemla
eBook ISBN: 9780323148153
Imprint: Academic Press
Published Date: 6th February 1987
Page Count: 496
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Description

Nonlinear Optical Properties of Organic Molecules and Crystals, Volume 1 discusses the nonlinear optical effects in organic molecules and crystals, providing a classical distinction between quadratic and cubic processes.

This book begins with a general overview of the basic properties of organic matter, followed by a review on the benefits derived from quantum-chemistry-based models and growth and characterization of high quality, bulk organic crystals and waveguided structures. A case study focusing on a specific material, namely urea, which exemplifies a situation in which transparency in the UV region has been purposely traded for nonlinear efficiency is also deliberated. This text concludes with a description of a type of trade-off between the unpredictable orientation of molecules in crystalline media, polarity of liquid-crystalline structures, and dominant electronic contribution to the electro-optic effect.

This publication is beneficial to solid-state physicists and chemists concerned with nonlinear optical properties of organic molecules and crystals.

Table of Contents


Preface: New Materials for a New Age


Part I. Introduction


Chapter I-1 The Structure and Properties of the Organic Solid State


I. Introduction


II. Structure


III. Electronic States


IV. Electronic Structure of Conjugated Polymers


V. Conclusion


References


Part II. Quadratic Nonlinear Optical Effects


Chapter II-1 Quadratic Nonlinear Optics and Optimization of the Second-Order Nonlinear Optical Response of Molecular Crystals


I. Introduction


II. Basic Concepts in Quadratic Nonlinear Optics


III. Second-Order Nonlinear Optical Effects


IV. Quadratic Nonlinear Effects in Organic Molecules


V. Relationships Between Microscopic and Macroscopic Optical Nonlinearities


VI. Nonlinear Organic Crystals: From Bulk to Waveguided Demonstration


VII. Conclusion


References


Chapter II-2 Molecular Hyperpolarizabilities of Organic Materials


I. Introduction


II. Electric-Field-Induced SHG in Liquids and Solutions


III. The Sum Over States Method


IV. Molecular Orbital Calculations of the Hyperpolarizability


V. The β Tensor for 4-Nitroaniline


VI. Calculations for Other Molecules


References


Chapter II-3 Design and Synthesis of Organic Molecular Compounds for Efficient Second-Harmonic Generation


I. Introduction


II. Origins of Optical Nonlinearity in Organic Molecular Crystals


III. Molecular Engineering


IV. Extensively Studied Organic Materials


V. Less Thoroughly Studied Organic Materials


VI. Conclusion


Details

No. of pages:
496
Language:
English
Copyright:
© Academic Press 1987
Published:
Imprint:
Academic Press
eBook ISBN:
9780323148153

About the Editor

D.S. Chemla

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